Arnim was a biochemist and genetic engineer who worked with the Nazis during World War II. There were plenty of rumours regarding an appearance from Arnim Zola before the series ever debuted, and he does have strong ties to both Captain America and Bucky. The human form of the Nazi/HYDRA scientist, Arnim Zola featured in last years Captain America: First Avenger movie where he was played by actor Toby Jones. TV Show: Ultimate Spider-Man Franchise: Spider-Man Number of Comparisons: 4 Franchise: Captain America Arnim Zola is a Marvel Comics supervillain who first appeared in Captain America #208 (Apr 1977). Cap's Arnim Zola Cast. Arnim Zola (Toby Jones) has died twice now in the Marvel Cinematic Universe, but is anyone ever really dead in the world of comic books? Mark Hamill is the voice of Arnim Zola in Lego Marvel Avengers. Mark Hamill is the voice of Arnim Zola in Ultimate Spider-Man, and Kotaro Nakamura is the Japanese voice. Arnim Zola Comparison of the voice actors who have been the voice of Arnim Zola with sound clips and images. The … After his brain upload, he appeared on monitors as green coding matching his face. Lego Marvel's Avengers (Video Game 2016) cast and crew credits, including actors, actresses, directors, writers and more. Video Game: Lego Marvel Avengers Franchise: Marvel Universe He frequently wore a Nazi outfit with a fedora as well as a scientist garb when doing scientist work. Toby Jones as Arnim Zola in Captain America: The First Avenger (Image credit: Marvel Studios) Who is Arnim Zola? He first appears in Captain America: The First Avenger as a scientist working for Hydra and the Red Skull before getting captured and recruited into S.H.I.E.L.D. Harry Potter actor joins the cast of Captain America. 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